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Effect of Ligand-Functionalized Enmeshed Metal-Organic Framework on Electrocatalytic Methanol Oxidation over O2 Reduction. The effect of ligand-functionalized metalloproteins on O2 reduction and methoxide generation in an enmeshed metal-organic framework (MOF) system was investigated. Three MOFs, namely, [Cu2(1,4-naphthalenedicarboxylic acid)2(4,4′-bipyridine)]2 (M-1) containing CuII ions and 4,4′-bipyridine (bipy) as ligands, [Co(1,4-naphthalenedicarboxylic acid)2(4,4′-bipyridine)]2 (M-2) containing CoII ions and bipy, and [Fe(1,4-naphthalenedicarboxylic acid)2(bipy)]2(FeII) (M-3) containing FeII ions and bipy, were chosen as model metal-containing MOFs for investigation. It was found that the catalytic activity of M-1 and M-2 were much higher than that of M-3. Apparently, the catalytic oxidation of methanol over M-1 and M-2 follows a similar catalytic cycle to that of the enzyme. In the electrocatalytic process, M-1 and M-2 exhibits better electrocatalytic properties than M-3. In addition, the M-1 and M-2 systems showed higher catalytic activities than the free ligands. Molecular simulations were further performed to elucidate the relationship between the structure of the enmeshed MOF and its electrocatalytic activity.Hilary Sampey Hilary Sampey (born March 24, 1972) is a Canadian former competition swimmer who won a bronze medal in the 4 × 100 m freestyle relay at the 1989 FINA World Aquatics Championships. Sampey was born in Hamilton, Ontario. She grew up in Tillsonburg, Ontario. Her father is a water polo official and her mother is a teacher. She attended Upper Canada College. See also List of University of Florida alumni References Category:1972 births Category:Living people Category:Canadian female freestyle swimmers Category:Sportspeople from Hamilton, Ontario Category:
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